CORDIS Project
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This project focuses on developing new types of chemical pairs called frustrated radical pairs for activating small molecules. By designing photoactivated versions of these pairs, the research aims to explore their potential in catalytic applications, particularly in bond activation reactions.
In 2006 Douglas Stephan described the first reversible metal-free hydrogen activation via frustrated Lewis pairs (FLPs).
In these pairs, the presence of bulky substituents in both the Lewis acid and base precludes the formation of the Lewis pair, creating a highly polarised pocket that can activate small and organic molecules.
Although mostly of the FLPs seem to react via two electron processes, a few FLPs have shown radical reactivity, namely frustrated radical pair (FRP).
This radical reactivi…
UNIVERSIDAD DE SEVILLA
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