CORDIS Project
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This project focuses on developing a method for meta carbonylative C-H acylation of arenes, which allows for the efficient synthesis of complex organic compounds. It aims to activate and carbonylate meta C-H bonds using transient directing groups and continuous flow techniques.
Carbonylative C-H activations can lead to an unprecedented degree of molecular sophistication by combining the atom-economical insertion of CO with the green activation of unreactive C-H bonds.
In striking contrast to ortho C-H acylation of arenes and heteroarenes (directing-group strategy) and para C-H ones (Friedel-Crafts chemistry), meta C-H acylations are almost completely unexplored.
This proposal aims at the development of the first example of meta C-H acylation via mild carbonylation of a…
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