CORDIS Project
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This project focuses on developing trifunctional catalytic systems that enable the selective functionalization of amides through innovative photocatalytic methods. By combining chiral hydrogen bonding with transition metal catalysis, the project aims to enhance the efficiency and variety of chemical reactions involving…
The trifunctional catalytic systems (TCS) consisting of bifunctional photocatalysts and transition metals will be designed to achieve the enantioselective N- C(sp3)-H functionalization of amides (ENCHFA).
Mechanistically, the bifunctional chiral hydrogen bonding-based aryl ketones will activate the amides to form -amido radicals via HAT and control their reactivity in an enantioselective manner while transition metal will provide another opportunity to active substrates and accomplish the photoc…
TECHNISCHE UNIVERSITAET MUENCHEN
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