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The Cu-CATARMs project aims to create an artificial metalloenzyme with a copper(I) center to enable new chemical transformations in a protein environment. This research focuses on developing methodologies for asymmetric reactions and understanding the underlying mechanisms of these processes.
The proposal that Cu-CATARMs (Asymmetric Copper(I) Catalysis in Artificial Metalloenzymes) aims to design and develop a proficient artificial metalloenzyme which contains a low oxidation state copper (Cu(I)) center, enabling a series of enantioselective new-to-nature transformations in a protein environment.The Roelfes group has been engaged in creation of LmrR based ARMs for the asymmetric copper-catalyzed new-to-nature reactions.
Reliable approaches have been developed by the Roelfes group to…
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