CORDIS Project
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This project focuses on developing a new chemical method for synthesizing dihydropyridinones through a cyclization cascade. The goal is to optimize this process for creating complex natural products with potential applications in cancer treatment.
During the course of this Fellowship a reductive cyclization cascade for dihydropyridinones, which consists of an iridium-catalyzed reduction to the corresponding electron-rich dienes and subsequent [4+2] cycloaddition (Diels-Alder reaction) will be developed.
A first promising proof of concept study establishing the feasibility of this powerful transformation has already been carried out in the Dixon group; however further optimization by varying the solvent, the reaction time, the temperature…
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