CORDIS Project
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This project investigates non-covalent interactions in large gas-phase molecular ions using infrared spectroscopy. By measuring frequency shifts related to molecular conformations, it aims to enhance understanding of dispersion forces, which are crucial for developing catalysts and materials.
We use IR spectroscopy of trapped ions in a cryogenic FT-ICR spectrometer to probe non-covalent, “dispersion” interactions in large, gas-phase molecular ions.
We will measure conformational equilibria by N-H frequency shifts, and correlate gas-phase IR frequency to the N-H-N bond angle in an ionic H-bond.
Substituents on “onium” cations can adopt various conformations, whose energies map interaction potentials.
Substituents on their proton-bound dimers interact non-covalently through dispersi…
EIDGENOESSISCHE TECHNISCHE HOCHSCHULE ZUERICH
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