CORDIS Project
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This project aims to create an artificial metalloenzyme using a dirhodium active site within a protein scaffold. The enzyme is designed to catalyze various chemical reactions relevant to the synthesis of pharmaceuticals and natural products under mild conditions.
Artificial metalloenzymes are expected to bring together the best of the two worlds of homogeneous and enzyme catalysis, combining broad substrate scope with high activity and reaction selectivity under mild conditions.
Herein we propose to construct an artificial metalloenzyme based on a dirhodium active site in the capsid scaffold of the protein ferritin.
Catalytically competent dirhodium compounds are derived from dirhodium tetraacetate, which possesses fourfold symmetry, with the ligands sym…
EIDGENOESSISCHE TECHNISCHE HOCHSCHULE ZUERICH
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